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25% - Efficiency flexible perovskite solar cells via controllable growth of SnO2 | TUP Journals & Magazine | IEEE Xplore

25% - Efficiency flexible perovskite solar cells via controllable growth of SnO2


Abstract:

High power conversion efficiency (PCE) flexible perovskite solar cells (FPSCs) are highly desired power sources for aerospace crafts and flexible electronics. However, th...Show More

Abstract:

High power conversion efficiency (PCE) flexible perovskite solar cells (FPSCs) are highly desired power sources for aerospace crafts and flexible electronics. However, their PCEs still lag far behind their rigid counterparts. Herein, we report a high PCE FPSC by controllable growth of a SnO2 electron transport layer through constant pH chemical bath deposition (CBD). The application of SnSO4 as tin source enables us to perform CBD without strong acid, which in turn makes it applicable to acid-sensitive flexible indium tin oxide. Furthermore, a mild and controllable growth environment leads to uniform particle growth and dense SnO2 deposition with full coverage and reproducibility, resulting in a record PCE of up to 25.09% (certified 24.90%) for FPSCs to date. The as-fabricated FPSCs exhibited high durability, maintaining over 90% of their initial PCE after 10000 bending cycles.
Published in: iEnergy ( Volume: 3, Issue: 1, March 2024)
Page(s): 39 - 45
Date of Publication: 22 March 2024
Electronic ISSN: 2771-9197

Funding Agency:

Department of Electrical Engineering, State Key Laboratory of Power System Operation and Control, Tsinghua University, Beijing, China
Department of Electrical Engineering, State Key Laboratory of Power System Operation and Control, Tsinghua University, Beijing, China
Department of Electrical Engineering, State Key Laboratory of Power System Operation and Control, Tsinghua University, Beijing, China
Department of Electrical Engineering, State Key Laboratory of Power System Operation and Control, Tsinghua University, Beijing, China
Department of Electrical Engineering, State Key Laboratory of Power System Operation and Control, Tsinghua University, Beijing, China
Department of Electrical Engineering, State Key Laboratory of Power System Operation and Control, Tsinghua University, Beijing, China
Center for Excellence in Nanoscience (CAS), Key Laboratory of Nanosystem and Hierarchical Fabrication (CAS), National Center for Nanoscience and Technology, Beijing, China
Department of Electrical Engineering, State Key Laboratory of Power System Operation and Control, Tsinghua University, Beijing, China

Department of Electrical Engineering, State Key Laboratory of Power System Operation and Control, Tsinghua University, Beijing, China
Department of Electrical Engineering, State Key Laboratory of Power System Operation and Control, Tsinghua University, Beijing, China
Department of Electrical Engineering, State Key Laboratory of Power System Operation and Control, Tsinghua University, Beijing, China
Department of Electrical Engineering, State Key Laboratory of Power System Operation and Control, Tsinghua University, Beijing, China
Department of Electrical Engineering, State Key Laboratory of Power System Operation and Control, Tsinghua University, Beijing, China
Department of Electrical Engineering, State Key Laboratory of Power System Operation and Control, Tsinghua University, Beijing, China
Center for Excellence in Nanoscience (CAS), Key Laboratory of Nanosystem and Hierarchical Fabrication (CAS), National Center for Nanoscience and Technology, Beijing, China
Department of Electrical Engineering, State Key Laboratory of Power System Operation and Control, Tsinghua University, Beijing, China

References

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