Enhanced Magnetostatic and Magnetodynamic Properties in Fe/Co Substituted Ni–Mn–In Alloy Films

The effects of the partial substitution of Mn by Co/Fe on the structural, magnetostatic, and magnetodynamic properties of Ni-Mn-In Heusler alloy films were studied using X-ray diffraction, field-dependent magnetization, and ferromagnetic resonance studies. It was observed that the substitution of up to 3 at.% Co or Fe atoms in Mn sites does not alter the crystal structure much. However, an increase in grain size and surface roughness was noticed upon substitution of the fourth element. The magnetic moment of the films could be increased up to 120 kA/m by introducing Co/Fe in Mn sites. For the first time, low Gilbert damping constant (α) of 0.008 is observed in Co substituted Ni-Mn-In film together with high saturation magnetization, high perpendicular anisotropy, and an easy axis along film plane, which are the promising factors for application in high-density random-access memory devices.