Frequency comb-assisted QCL stabilization for high resolution molecular spectroscopy

We present a frequency comb-assisted experimental setup which enables us to both coherently transfer the stability and accuracy of a remote near-infrared (NIR) ultrastable laser to a mid-infrared (MIR) quantum cascade laser (QCL), and widely tune the QCL frequency for spectroscopic applications. The QCL is stabilized at the level of 2×10
⁻¹⁵
from 1 to 100 s, with an accuracy of 10
⁻¹⁴
after 100 s. The achievable frequency tuning paves the way for high-resolution saturated absorption spectroscopy of molecular transitions, in particular in spectral regions that were previously inaccessible with standard stabilized MIR lasers. Preliminary results show a sensitivity at the kHz level on transition center frequencies.