Measurement of Equilibrium Spin Polarization in Spin-Exchange Relaxation-Free Atomic Magnetometers via the Steady-State Response to the Triaxial Magnetic Field

This study proposes an in situ method for measuring the equilibrium spin polarization and its longitudinal spatial distribution in a spin-exchange relaxation-free (SERF) atomic magnetometer. The total relaxation rate was determined by analyzing the steady-state response of the magnetometer to the triaxial magnetic field. The transfer coefficient between spin polarization along the probe beam axis and the steady-state response was derived from the optical depth of the probe light and the incident/transmitted power through the vapor cell. By applying a DC magnetic field along the sensitive axis and combining the total relaxation rate with the transfer coefficient, the equilibrium spin polarization value under zero-field conditions was obtained. The equilibrium spin polarization distribution along the pump beam propagation direction was measured, showing consistent trends with simulation results, with a maximum relative error of less than 5%. The expanded uncertainty of the proposed equilibrium spin polarization measurement method ranges from 0.8% to 9.7%. The advantages of this method include no requirement for additional optical field or magnetic field modulation, immunity to temperature and temperature gradients, and the capability to directly determine the equilibrium spin polarization value.