Investigation on Thermal Characteristics and Performance of Cylindrical Lithium-Ion Battery Pack Using P2D Model With Varied Electrode Chemistries

Efficient heat dissipation in lithium-ion battery packs is crucial for safety, necessitating a thorough assessment of thermal performance during the design phase. This study utilizes Newman’s Pseudo two-dimensional (P2D) model and three-dimensional computational fluid dynamics to depict heat generation and dissipation. The main objectives include evaluating heat dynamics, establishing optimal temperature limits, and assessing State of Charge (SOC) and State of Health (SOH) estimations. The battery pack, configured in 6s2p, features plastic-wrapped cylindrical modules with air-filled domains, connected in parallel pairs with aluminum wires. Active materials comprise positive electrodes like Lithium Cobalt Oxide (LCO), Lithium Nickel Manganese Cobalt Oxide (NMC), Lithium Iron Phosphate (LFP), and Lithium Manganese Oxide (LMO), with graphite as the negative electrode and a separator (Lithium Hexa Fluoro Phosphate). Results indicate that air-cooled NMC electrode chemistry achieves a peak heat dissipation of 102.48W, maintaining an optimal temperature range of 21.3deg C to 32.8deg C. After 1000 cycles, the optimal temperature limit of 32.8deg C with an 80% capacity loss minimizes negative impacts during charge/discharge cycles. SOC and SOH remain at 100% and 80%, utilizing an 8Ah battery with a nominal voltage of 4.2V, and a 3.9-year life expectancy, addressing charge/discharge cycle issues.