Ultrafast Orbital Tomography of a Molecular Film at a FEL

Understanding and control of photon-induced dynamics of molecules on solid surfaces are of essential importance for surface chemistry as well as for design of novel devices. In the last decade, orbital tomography has emerged as an exciting extension of the photoemission technique for imaging the wave functions of molecules in thin films [1]. Extending this technique into the time domain will provide unprecedented insight into photon-induced dynamics and chemical reactions [2].