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Second-harmonic generation properties of 2-amino-5-nitropyridinium-dihydrogenarsenate and -dihydrogenphosphate organic-inorganic crystals

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6 Author(s)
Feve, J.P. ; Lab. de Phys. du Solide, Bourgogne Univ., Dijon, France ; Boulanger, B. ; Rousseau, I. ; Marnier, G.
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We present a comparative study of the linear and nonlinear optical properties of two isomorphous organic-inorganic crystals: the 2-amino 5-nitropyridinium-dihydrogenphosphate (2A5NPDP) and -dihydrogenarsenate (2A5NPDAs). We determine accurate equations for the dispersion in wavelength of their principal refractive indices from direct prism measurements and from angular noncritically phase-matched second-harmonic generation (SHG) experiments. We deduce the quadratic nonlinear coefficients d15 and d24 of each compound from the phase-matched conversion efficiency of SHG experiments and find that they are close to those of KTiOPO4

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Quantum Electronics, IEEE Journal of  (Volume:35 ,  Issue: 1 )