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In this paper are described measurements at high-altitude of both radiation environment and effects. These measurements comprise cosmic ray neutrons and SBU/MCU on nanoscales devices. Results obtained at Pic-du-Midi, France, and in the city of Puno, Peru, are presented and analyzed. Analyses and cross comparisons based-on MUSCA SEP3 calculations show a good agreement between experimental data and modeling, thus illustrating the importance of the knowledge of the radiation field for a reliable prediction.