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This paper presents the system design method to determine the modulation and coding schemes according to the given usage models of single carrier transmission in millimeter wave Wireless LAN systems. Various modulation and coding combinations are compared and analyzed based on the BER performance over both AWGN and fading channels. The effects of hardware impairments including power amplifier non-linear effects and phase noise, etc., are considered as well. The system design strategy provides a guideline for the selection of modulation and coding schemes in practical which can fulfill the realistic system requirements.