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Structural, magnetic, electrical transport properties, and reversible room-temperature magnetocaloric effect in antipervoskite compound AlCMn3

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10 Author(s)
Wang, B.S. ; Key Laboratory of Materials Physics, Institute of Solid State Physics, Hefei 230031, People’s Republic of China ; Lin, J.C. ; Tong, P. ; Zhang, L.
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We report the structural, magnetic, electrical transport properties, and magnetocaloric effect (MCE) of antipervoskite compound AlCMn3. It exhibits a second-order ferromagnetic–paramagnetic phase transition around (TC) 287 K. The electronic resistivity (ρ) shows a good metallic behavior except for a slope change around TC. At lower temperatures (below 130 K), ρ∝T2 indicates that the electron-electron scatterings domain. At evaluated temperatures (130–270 K), ρ is linear dependence on temperature, implying that the phonon scatterings boost up greatly. Furthermore, a broad distribution of the magnetic entropy change (-ΔSM) peak is found to about 100 K with the magnetic field change ΔH=45 kOe. The relative cooling power are ∼137 J/kg and ∼328 J/kg (or ∼68 K2 and ∼162 K2) with ΔH=20 kOe and 45 kOe, respectively. All these values are comparable with the typical MCE associated with a second-order transition. It suggests that AlCMn3 may be considered as a candidate material for near room-temperature magnetic refrigeration because of: (i) the large full width at half peak of the -ΔSM-T curve, (ii) no hysteresis losses, (iii) the near room-temperature working temperature, and (iv) the low-cost and innoxious raw materials. Moreover, it is foun- - d that the simple theoretical model which only considering the magnetoelastic and magnetoelectronic couplings couldn’t account well for the observed MCE in antiperovskite AlCMn3.

Published in:

Journal of Applied Physics  (Volume:108 ,  Issue: 9 )