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Single crystal-like selection rules for unipolar-axis oriented tetragonal Pb(Zr,Ti)O3 thick epitaxial films

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10 Author(s)
Nakajima, Mitsumasa ; Department of Innovative and Engineered Materials, Tokyo Institute of Technology, Yokohama 226-8502, Japan ; Fujisawa, Takashi ; Ehara, Yoshitaka ; Yamada, Tomoaki
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We investigated the polarized Raman spectra of a strain-free, unipolar-axis oriented tetragonal Pb(Zr,Ti)O3 thick epitaxial film. We evaluated the single crystal-like selection rules of the A1- and E-symmetry components, and found an anomalous behavior in the angular dependence of the A1(1TO)-mode intensity similar to that observed in high-Tc superconductor single crystals. Raman tensor analyses of the A1(1TO) mode revealed complex phases may exist between two independent Raman-tensor components even in the single 180° domain state.

Published in:

Applied Physics Letters  (Volume:97 ,  Issue: 11 )

Date of Publication:

Sep 2010

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