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Abnormal behavior of supercooled liquid region in bulk-forming metallic glasses

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3 Author(s)
Park, E.S. ; Department of Materials Science and Engineering, Research Institute of Advanced Materials, Seoul National University, Seoul 151-744 Republic of Korea ; Na, J.H. ; Kim, D.H.

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A metallic glass is often viewed as an amorphous alloy exhibiting a single endothermic reaction in the supercooled liquid region (SCLR, ΔTx=Tx-Tg). Here we discuss the origin and consequences of abnormal behavior of SCLR in various bulk-forming metallic glasses (BMGs). The two-stage-like endothermic reaction in Ni-based, Cu-based, Zr-based, and Mg-based BMGs can originate from the local immiscibility of liquids, which is closely related to chemical heterogeneity in as-cast BMG. These inflections can be attributed to the overlap of the exothermic reaction for the formation and growth of clusters in SCLR. The abnormal behavior of SCLR can be modulated by controlling cooling rate as well as by tailoring alloy composition, with the consequence that the modulated local heterogeneity in these BMGs can lead to enhanced flexibility of the BMGs. This correlation assists in understanding toughening mechanism and in guiding alloy design to alleviate brittleness of BMGs.

Published in:

Journal of Applied Physics  (Volume:108 ,  Issue: 5 )