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Semiclassical theory and numerical modeling for stimulated rotational Raman scattering in homonuclear diatomic molecules

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3 Author(s)
Parazzoli, C. ; Hughes Aircraft Co., El Segundo, CA, USA ; Drutman, C. ; Capps, D.M.

The semiclassical theory of nonresonant stimulated rotational Raman scattering (SRRS) in homonuclear diatomic molecules has been developed. Multiple rotational lines, the full degeneracy of the molecule, Stark shift, and four-wave mixing effects are considered. An arbitrary number of optical fields is allowed. The polarization state of the fields is dynamically computed during the propagation. A numerical code has been written in a user-friendly format based on the theoretical model with diffractive effects included. Numerical results which display the code capabilities are presented and comparisons to available experimental data are shown

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Quantum Electronics, IEEE Journal of  (Volume:26 ,  Issue: 4 )