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Advantages of superconducting quantum interference device-detected magnetic resonance over conventional high-frequency electron paramagnetic resonance for characterization of nanomagnetic materials

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4 Author(s)
Cage, Brant ; National Institute of Standards and Technology, Boulder, Colorado 80305 ; Russek, Stephen E. ; Zipse, David ; Dalal, Naresh S.

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A dc-detected high-frequency electron paramagnetic resonance (HF-EPR) technique, based on a standard superconducting quantum interference device (SQUID) magnetometer, has significant advantages over traditional HF-EPR based on microwave absorption measurements. The SQUID-based technique provides quantitative determination of the dc magnetic moment as a function of microwave power, magnetic field and temperature. The EPR spectra obtained do not contain variability in the line shape and splittings that are commonly observed in the standard single-pass transmission mode HF-EPR. We demonstrate the improved performance by comparing EPR spectra for Fe8 molecular nanomagnets using both SQUID-based and conventional microwave-absorption EPR systems.

Published in:

Journal of Applied Physics  (Volume:97 ,  Issue: 10 )