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Dispersion and pulse-duration dependence of the nonlinear optical response of Gd2 at C80

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4 Author(s)
Yaglioglu, Gul ; Electrical Engineering Department, City College and Graduate Center of the City University of New York, New York, New York 10031 ; Pino, Robinson ; Dorsinville, Roger ; Liu, J.Z.

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Single-beam z-scan and transient absorption experiments were carried out between 400 and 1000 nm in Gd2 at C80 thin films and solutions. The third-order nonlinearity was large, negative, and strongly dependent on pulse duration and wavelength. Transient absorption results suggest that the fast nonlinear response is enhanced by two-photon-induced ground-state absorption and excited-state bleaching effects. © 2001 American Institute of Physics.

Published in:

Applied Physics Letters  (Volume:78 ,  Issue: 7 )

Date of Publication:

Feb 2001

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