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Fundamental optical absorption edge of undoped tetragonal zirconium dioxide

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3 Author(s)
Aita, C.R. ; Advanced Coatings Experimental Laboratory, University of Wisconsin-Milwaukee, P.O. Box 784, Milwaukee, Wisconsin 53201 ; Hoppe, E.E. ; Sorbello, R.S.

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The high-frequency optical absorption edge of pure tetragonal ZrO2, isolated in a ZrO2Al2O3 nanolaminate film structure, was determined using transmission spectrophotometry. The functional dependence of the absorption coefficient on photon energy shows two interband transitions: an initial indirect transition at 5.22 eV (i.e., the band gap) followed by a direct transition at 5.87 eV. The edge structure is associated with O 2p→Zr 4d electron states and discussed in terms of ab initio calculations reported in the literature. © 2003 American Institute of Physics.

Published in:

Applied Physics Letters  (Volume:82 ,  Issue: 5 )

Date of Publication:

Feb 2003

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