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Effect of misfit strain on the multiferroism and nonlinear optical response in epitaxial PbVO3 thin films

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2 Author(s)
Ju, Sheng ; Department of Physics, Soochow University, Suzhou 215006, China ; Cai, Tian-Yi

Your organization might have access to this article on the publisher's site. To check, click on this link:http://dx.doi.org/+10.1063/1.3050526 

Based on density functional theory (the generalized gradient approximation plus on-site Coulomb repulsion method), we investigate the misfit strain dependence of multiferroism and second-harmonic generation (SHG) in epitaxial PbVO3 thin films. G-type antiferromagnetic ordering, large polar distortion, and significant SHG susceptibilities are revealed in PbVO3 over a wide range of substrates. In particular, the low frequency SHG susceptibility reaches as high as 300×10-9 esu in all the cases we considered, providing solid evidence of its potential application in nonlinear optoelectronic device.

Published in:

Applied Physics Letters  (Volume:93 ,  Issue: 25 )

Date of Publication:

Dec 2008

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