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Generation of ultrashort optical pulses using multiple coherent anti-Stokes Raman scattering in a crystal at room temperature

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3 Author(s)
Matsubara, E. ; Department of Applied Physics, Hokkaido University, and Core Research for Evolutional Science and Technology (CREST), Japan Science and Technology Agency (JST), Kita-13, Nishi-8, Kita-ku, Sapporo 060-8628, Japan ; Sekikawa, T. ; Yamashita, M.

Your organization might have access to this article on the publisher's site. To check, click on this link:http://dx.doi.org/+10.1063/1.2883928 

We demonstrate Fourier synthesis of multiple coherent anti-Stokes Raman scattering signals in a LiNbO3 crystal at room temperature. The signals up to the 20th order (470–800 nm) were generated by two crossing femtosecond Ti:sapphire laser pulses. Angle dispersion of the signals was compensated into one white-continuum beam by modifying a conventional 4f configuration. Spectral phase of the signal was measured by spectral phase interferometry for direct electric-field reconstruction. Isolated pulses with 25 fs duration at 1 kHz were generated only by appropriately aligning the angle-dispersion compensator. This result opens the possibility of the generation of subfemtosecond pulses in the visible region.

Published in:

Applied Physics Letters  (Volume:92 ,  Issue: 7 )

Date of Publication:

Feb 2008

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