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Noncritical phase-matched lithium triborate optical parametric oscillator for high resolution coherent anti-Stokes Raman scattering spectroscopy and microscopy

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4 Author(s)
Jurna, M. ; Optical Techniques Groupb), Department of Science and Technology, MESA+ Institute for Nanotechnology, University of Twente, Enschede, Overijssel 7500 AE, The Netherlands ; Korterik, J.P. ; Offerhaus, H.L. ; Otto, C.

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An efficient, widely tunable, narrow-bandwidth, green-pumped, noncritical phase-matched lithium triborate based optical parametric oscillator (OPO) is applied to coherent anti-Stokes Raman scattering (CARS) spectroscopy and microscopy. The tunable signal beam (740–930 nm) of the OPO is combined with the fundamental of a Nd:YVO4 pump laser (1064 nm, 15 ps) to obtain high resolution vibrational spectra of molecules around the CH vibrational stretch (2700–3100 cm-1). The straightforward and convenient tunability of the OPO is demonstrated by CARS microscopy for the identification of different polymer microparticles on the same substrate.

Published in:

Applied Physics Letters  (Volume:89 ,  Issue: 25 )

Date of Publication:

Dec 2006

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