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Packing-induced electronic structure changes in bundled single-wall carbon nanotubes

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7 Author(s)
Castrucci, P. ; Dipartimento di Fisica, Unità INFM, Università di Roma “Tor Vergata”, Via della Ricerca Scientifica 1, 00133 Roma, Italy ; Scarselli, M. ; De Crescenzi, M. ; Diociaiuti, M.
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The electronic structure of free-standing parallel and braided bundles of single-wall carbon nanotubes (∼1.2 nm diameter) was probed by transmission electron microscopy and electron energy loss spectroscopy. The observed dramatic changes in the carbon K(1s) near-edge structures are attributed to the tubes’ structural packing in bundles which consequently alters their electronic structure. The π*- and the σ*-states are shown to be strongly affected by the way the tubes are packed in the bundles (i.e., parallel, braided, turned, or twisted).

Published in:

Applied Physics Letters  (Volume:87 ,  Issue: 10 )

Date of Publication:

Sep 2005

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