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In this study, the Bi3.9Ti2.9V0.08O12 (BTV) thin films have been well deposited on the Pt/Ti/SiO2/Si substrate. The optimum radio frequency (RF) deposition parameters of BTV thin films are developed, and they are RF power of 130 W, substrate temperature of 550degC, chamber pressure of 10 m Torr, and oxygen concentration of 25 %. As the applied voltage is increased to 10 V, the remnant polarization and coercive field of BTV thin films are about 3.8 muC/cm2 and 220 kV/cm. The counterclockwise current hysteresis and memory window of non-volatile FeRAM devices property are observed, and that can be used to indicate the switching effect of ferroelectric polarization of BTV thin films. Finally, the BTV FeRAM devices with channel width = 40 mum and channel length = 20 mum has been successfully fabricated and the ID-VG transfer characteristics are also investigated in this study.