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This paper proposes an approach of cooperative control that is based on the concept of combining neural networks and the methodology of sliding mode control (SMC). The main purpose is to eliminate the chattering phenomenon. Next, the system performance can be improved by using the method of SMC. In the present approach, two parallel Neural Networks are utilized to realize a neuro-sliding mode control (NSMC), where the equivalent control and the corrective control are the outputs of neural network 1 and neural network 2, respectively. Based on expressions of the SMC, the weight adaptations of neural network can be determined. Furthermore, the gradient descent method is used to minimize the control force so that the chattering phenomenon can be eliminated. Finally, experimental results are given to show the effectiveness and feasibility of the approach.