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Ellipse rotation studies in laser host materials

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1 Author(s)
Owyoung, Adelbert ; Sandia Laboratories, Albuquerque, NM, USA

Using a TEM00qnear Gaussian mode ruby laser system we report the first experimental measurements of intensity induced changes of optical polarization (ellipse rotation) in a cubic crystalline medium, YAG, for which we obtain the nonlinear susceptibilitieschi_{3}^{1221} (- omega, omega, omega, -omega) = 6.34 times 10^{-15}ESU andfrac{1}{2} (chi_{3}^{1111} + chi_{3}^{1221} - 2chi_{3}^{1212}) = 7.18 times 10^{-15}ESU, accurate to better than ±7 percent relative tochi_{3}^{1221} (- omega,omega,omega, -omega)for liquid CS2. These values are compared with further results obtained for fused quartz and two laser glasses. Moreover, by time resolving the ellipse rotation data we demonstrate the capability to plot ellipse rotation versus input power on a single laser shot, thus increasing the practical feasibility of the technique and introducing the possibility of resolving transient contributions to the measurement.

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Quantum Electronics, IEEE Journal of  (Volume:9 ,  Issue: 11 )