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1C4 - Infrared difference frequency generation

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2 Author(s)
Martin, M. ; Ministry of Aviation, Signals Research and Developement, Christchurch, Hampshire, England ; Thomas, E.

Several molecular vibrational frequencies have been generated by beating together a laser and laser-stimulated Raman emission. A Nd3+/glass laser was used to excite Raman emission from C6H6, C6D6, and CH3. NO2. The difference frequencies were generated in a single crystal of CdS and appeared at 992, 944, and 927 cm-1, respectively. A difference frequency has also been detected at 944 cm-1following mixing in CdSe. The data presented for HgS indicates that phase-matched outputs can be generated over a limited range of frequencies, provided that the Raman emission is excited with a Nd3+/glass laser. Experimental details are given and the results are discussed.

Published in:

Quantum Electronics, IEEE Journal of  (Volume:2 ,  Issue: 8 )

Date of Publication:

August 1966

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