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Limitation of 3547 to 1182 Å conversion efficiency in Xe

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2 Author(s)
Zych, L. ; Stanford University, Stanford, CA, USA ; Young, J.

We report experiments which indicate that the 3547 → 1182Å conversion efficiency in Xe-Ar mixtures is limited by Kerr-induced dispersion to about 0.9 percent. The mixed frequency third-order nonlinearity \chi ^{(3)}(-3\omega , 3\omega , -\omega , \omega ) significantly alters the index of refraction at 1182 Å in the presence of large power densities at 3547 Å, affecting phase matching. We suggest using a Xe-Mg-Ar mixture to reduce the effect, thus permitting increased efficiencies.

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Quantum Electronics, IEEE Journal of  (Volume:14 ,  Issue: 3 )